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Wood Science and Technology

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12.11.2022 | Original

In situ growth of bimetallic Co/Zn-ZIF within wood scaffold for enhanced adsorption capacity and improved flame retardancy

verfasst von: Gang Zhu, Hui Li, Shuduan Deng, Chaoling Zhang, Kunyong Kang, Xupeng Zhang, Kaiqian Li

Erschienen in: Wood Science and Technology | Ausgabe 6/2022

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Abstract

Metal–organic frameworks (MOFs)/wood are attractive hybrid materials that offer a range of multifunctional properties by integrating MOFs into wood substrates. Although a good foundation has been laid in studies, it is clear that studies are limited to the conjugation of wood with monometallic MOFs. Research on the utility of novel hybrid materials designed incorporating bimetallic MOFs into wood has not yet been encountered. Herein, a novel bimetallic cobalt/zinc-based zeolite imidazolate frameworks (Co/Zn-ZIF)@wood hybrid material was successfully fabricated through in situ growth of Co-ZIF-67 and Zn-ZIF-8 within balsa wood channel arrays. SEM images indicated that Co/Zn-ZIF exhibited smaller particle sizes compared with Co and Zn monometallic MOFs. The resulting composite displays high removal efficiency up to 97.2% for methylene blue and the adsorption capacity can reach 223.6 mg·g⁻¹ at 298 K. Moreover, the incorporation of Co/Zn-ZIF has better effect on thermal stability at the early stage and char layer formatting of wood substrate than monometallic MOFs. Compared with the monometallic MOF additives, the peak of heat release rate of the Co/Zn-ZIF@wood hybrid materials exhibited a drastic decline by 67.5% from 94.5 to 30.7 W·g⁻¹ and the total heat release from 7.7 to 3.5 kJ·g⁻¹. In addition, the introduction of Co/Zn-ZIF increases the limiting oxygen index (LOI) values of the prepared composites, and the treated wood had a strong self-extinguishing ability, which manifested that Co/Zn-ZIF@wood had excellent flame retardancy. This work offers a new avenue for designing and constructing functionalized MOFs@wood composites that may boost their environmental- and green building-related applications.

Vorheriger Artikel Shear traction‐separation laws of European beech under mode II loading by 3D digital image correlation

Nächster Artikel Effects of molecular weight of urea–formaldehyde resins on wettability and adhesion at wood surface, interphase, and plywood

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Titel: In situ growth of bimetallic Co/Zn-ZIF within wood scaffold for enhanced adsorption capacity and improved flame retardancy
verfasst von: Gang Zhu
Hui Li
Shuduan Deng
Chaoling Zhang
Kunyong Kang
Xupeng Zhang
Kaiqian Li
Publikationsdatum: 12.11.2022
Verlag: Springer Berlin Heidelberg
Erschienen in: Wood Science and Technology / Ausgabe 6/2022
Print ISSN: 0043-7719
Elektronische ISSN: 1432-5225
DOI: https://doi.org/10.1007/s00226-022-01430-w

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